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The interaction between silica flat substrate and functional group-modified nanoparticles
X. H. He; L. Y. Deng; L. Y. Shi; Y. B. Deng; T. Zhou and L. P. Wen
2022
发表期刊Electrophoresis
ISSN0173-0835
卷号43期号:20页码:1984-1992
摘要Inspired by nature, the research of functionalized nanoparticles and nanodevices has been in-depth developed in recent years. In this paper, we theoretically studied the interaction between functional polyelectrolyte brush layer-modified nanoparticles and a silica flat substrate. Based on the Poisson-Nernst-Planck equations, the mathematical model is established. The changes of the volume charge density and electric field energy density when the nanoparticle interacts with the silica flat substrate under multi-ions regulation were investigated. The results show that when there is a strong interaction between the silica flat substrate and nanoparticles, such as the distances between the nanoparticle and silica flat substrate, which are 2 or 5 nm, the isoelectric point shift under the influence of silica flat substrate and the total charge density in the brush layer is jointly controlled by the cations in the solution and the volume charge density of the brush layer. With the increase of the distances between the nanoparticle and silica flat substrate, the regulation of the volume charge density of the brush layer dominates. These results will provide guidance for the movement mechanism of functionalized nanoparticles in silica nanochannels.
DOI10.1002/elps.202100262
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收录类别sci
语种英语
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被引频次:2[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/66765
专题中国科学院长春光学精密机械与物理研究所
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X. H. He,L. Y. Deng,L. Y. Shi,et al. The interaction between silica flat substrate and functional group-modified nanoparticles[J]. Electrophoresis,2022,43(20):1984-1992.
APA X. H. He,L. Y. Deng,L. Y. Shi,Y. B. Deng,&T. Zhou and L. P. Wen.(2022).The interaction between silica flat substrate and functional group-modified nanoparticles.Electrophoresis,43(20),1984-1992.
MLA X. H. He,et al."The interaction between silica flat substrate and functional group-modified nanoparticles".Electrophoresis 43.20(2022):1984-1992.
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