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Effects of annealing temperature, thickness and substrates on optical properties of m-plane ZnO films studied by photoluminescence and temperature dependent ellipsometry
Y. Liu,T. Y. He,D. H. Chen,H. Yang,I. T. Ferguson,D. Huang and Z. C. Feng
2020
发表期刊Journal of Alloys and Compounds
ISSN0925-8388
卷号848页码:10
摘要A series of m-plane ZnO films grown on sapphire and Si substrates with different thicknesses (186-371 nm) and different annealing temperatures (150-200 degrees C) were studied in detail by comparing X-ray diffraction, photoluminescence and spectroscopic ellipsometry measurements. The impact of thickness, annealing temperature and substrates on optical properties was investigated by the systematical analysis of the highly correlated stain, grain size, exciton effect, absorption tailing and crystallinity. Our finding indicates that the improvement of crystal quality along with the increase of grain size and refractive index for m-plane ZnO can be observed with increasing annealing temperature, increasing thickness or by introducing sapphire instead of Si substrate. The refractive index and bandgap have stronger dependence on annealing temperature than on thickness, causing the blue-shift of bandgap with rising annealing temperature despite thicker film. This bandgap shift is more pronounced for ZnO in ZnO/Si system. Photoluminescence combined with ellipsometry analysis demonstrate that higher annealing temperature can strengthen the excitonic feature. Bose-Einstein equation, employed to fit the dependence of bandgap on experimental temperature (300-583 K) illustrates that, the reduction of bandgap at elevated temperatures is more significant for ZnO in ZnO/sapphire system due to the corresponding stronger electron/exciton-phonon interactions involved with larger longitudinal optical phonon energies. (C) 2020 Elsevier B.V. All rights reserved.
DOI10.1016/j.jallcom.2020.156631
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收录类别SCI ; EI
语种英语
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文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/64478
专题中国科学院长春光学精密机械与物理研究所
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Y. Liu,T. Y. He,D. H. Chen,H. Yang,I. T. Ferguson,D. Huang and Z. C. Feng. Effects of annealing temperature, thickness and substrates on optical properties of m-plane ZnO films studied by photoluminescence and temperature dependent ellipsometry[J]. Journal of Alloys and Compounds,2020,848:10.
APA Y. Liu,T. Y. He,D. H. Chen,H. Yang,I. T. Ferguson,D. Huang and Z. C. Feng.(2020).Effects of annealing temperature, thickness and substrates on optical properties of m-plane ZnO films studied by photoluminescence and temperature dependent ellipsometry.Journal of Alloys and Compounds,848,10.
MLA Y. Liu,T. Y. He,D. H. Chen,H. Yang,I. T. Ferguson,D. Huang and Z. C. Feng."Effects of annealing temperature, thickness and substrates on optical properties of m-plane ZnO films studied by photoluminescence and temperature dependent ellipsometry".Journal of Alloys and Compounds 848(2020):10.
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