Changchun Institute of Optics,Fine Mechanics and Physics,CAS
Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer | |
Q. Li; X. Xie; H. Wu; H. Chen; W. Wang; X. Kong and Y. Chang | |
2023 | |
发表期刊 | Nano Letters
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ISSN | 15306984 |
卷号 | 23期号:8页码:3444-3450 |
摘要 | Highly doped lanthanide luminescent nanoparticles exhibit unique optical properties, providing exciting opportunities for many ground-breaking applications, such as super-resolution microscopy, deep-tissue bioimaging, confidentiality, and anticounterfeiting. However, the concentration-quenching effect compromises their luminescence efficiency/brightness, hindering their wide range of applications. Herein, we developed a low-temperature suppression cross-relaxation strategy, which drastically enhanced upconversion luminescence (up to 2150-fold of green emission) in Er3+-rich nanosystems. The cryogenic field opens the energy transport channel of Er3+ multiphoton upconversion by further suppressing phonon-assisted cross-relaxation. Our results provide direct evidence for understanding the energy loss mechanism of photon upconversion, deepening a fundamental understanding of the upconversion process in highly doped nanosystems. Furthermore, it also suggests the potential applications of upconversion nanoparticles for extreme ambient-temperature detection and anticounterfeiting. © 2023 American Chemical Society. |
DOI | 10.1021/acs.nanolett.3c00495 |
URL | 查看原文 |
收录类别 | sci ; ei |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ciomp.ac.cn/handle/181722/67635 |
专题 | 中国科学院长春光学精密机械与物理研究所 |
推荐引用方式 GB/T 7714 | Q. Li,X. Xie,H. Wu,et al. Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer[J]. Nano Letters,2023,23(8):3444-3450. |
APA | Q. Li,X. Xie,H. Wu,H. Chen,W. Wang,&X. Kong and Y. Chang.(2023).Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer.Nano Letters,23(8),3444-3450. |
MLA | Q. Li,et al."Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer".Nano Letters 23.8(2023):3444-3450. |
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