中国科学院长春光学精密机械与物理研究所

QQ客服 官方微博 反馈留言

	Break through the Steric Hindrance of Ionic Liquids with Carbon Quantum Dots to Achieve Efficient and Stable Perovskite Solar Cells
	S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang
	2023
发表期刊	ACS Applied Materials and Interfaces
ISSN	19448244
卷号	15期号:41页码:48304-48315
摘要	Overcoming the negative impact of residual ionic liquids (ILs) on perovskite films based on an in-depth understanding of chemical interactions between ionic liquids and preparing perovskite precursor solutions is a great challenge when aiming to simultaneously achieve long-term stability and high efficiency within IL-based perovskite solar cells (PSCs). Herein, 1-butyl-3-methylimidazolium tetrafluoroborate (BMIMBF4), a type of IL, was introduced into the perovskite precursor solution, and carbon quantum dots (CQDs) were further introduced into the antisolvent to enhance the photovoltaic properties of PSCs. Both ILs and CQDs synergistically manipulate the crystallization process and passivate defects to obtain high-quality perovskite films. Besides serving as passivation sites to strengthen the collaboration between additives and perovskite materials, the cointroduction of CQDs further promotes the carrier transport process since it not only provides carrier channels at grain boundaries but also forms better energy alignment, which effectively overcomes the charge transfer loss caused by the steric hindrance of ILs. Based on such a synergistic effect of ILs and CQDs, the n-i-p MAPbI3-based PSCs achieve the highest efficiency of 20.84% with improved stability. This simple and low-cost synergistic integration method will subsequently provide direction for optimizing ILs to improve the photovoltaic performance of PSCs. © 2023 American Chemical Society
DOI	10.1021/acsami.3c11370
URL	查看原文
收录类别	sci ; ei
引用统计
文献类型	期刊论文
条目标识符	http://ir.ciomp.ac.cn/handle/181722/67408
专题	中国科学院长春光学精密机械与物理研究所
推荐引用方式 GB/T 7714	S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang. Break through the Steric Hindrance of Ionic Liquids with Carbon Quantum Dots to Achieve Efficient and Stable Perovskite Solar Cells[J]. ACS Applied Materials and Interfaces,2023,15(41):48304-48315.
APA	S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang.(2023).Break through the Steric Hindrance of Ionic Liquids with Carbon Quantum Dots to Achieve Efficient and Stable Perovskite Solar Cells.ACS Applied Materials and Interfaces,15(41),48304-48315.
MLA	S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang."Break through the Steric Hindrance of Ionic Liquids with Carbon Quantum Dots to Achieve Efficient and Stable Perovskite Solar Cells".ACS Applied Materials and Interfaces 15.41(2023):48304-48315.

条目包含的文件		下载所有文件
文件名称/大小	文献类型	版本类型	开放类型	使用许可
Break through the St（6420KB）	期刊论文	出版稿	开放获取	CC BY-NC-SA	浏览 下载

个性服务

推荐该条目

保存到收藏夹

查看访问统计

导出为Endnote文件

谷歌学术

谷歌学术中相似的文章

[S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang]的文章

百度学术

百度学术中相似的文章

[S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang]的文章

必应学术

必应学术中相似的文章

[S. Chi, S. Yang, Y. Wang, D. Li, L. Zhang, L. Fan, F. Wang, X. Liu, H. Liu, M. Wei, J. Yang and L. Yang]的文章

相关权益政策

暂无数据

收藏/分享

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。