Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance

doi:10.1002/aenm.202000453

CIOMP OpenIR

	Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance
	W. C. Kong; S. W. Wang; F. Li; C. Zhao; J. Xing; Y. T. Zou; Z. Yu; C. H. Lin; Y. W. Shan; Y. H. Lai; Q. F. Dong; T. Wu; W. L. Yu and C. L. Guo
	2020
发表期刊	Advanced Energy Materials
ISSN	1614-6832
卷号	10 期号:34 页码:8
摘要	Grains and grain boundaries play key roles in determining halide perovskite-based optoelectronic device performance. Halide perovskite monocrystalline solids with large grains, smaller grain boundaries, and uniform surface morphology improve charge transfer and collection, suppress recombination loss, and thus are highly favorable for developing efficient solar cells. To date, strategies of synthesizing high-quality thin monocrystals (TMCs) for solar cell applications are still limited. Here, by combining the antisolvent vapor-assisted crystallization and space-confinement strategies, high-quality millimeter sized TMCs of methylammonium lead iodide (MAPbI(3)) perovskites with controlled thickness from tens of nanometers to several micrometers have been fabricated. The solar cells based on these MAPbI(3)TMCs show power conversion efficiency (PCE) of 20.1% which is significantly improved compared to their polycrystalline counterparts (PCE) of 17.3%. The MAPbI(3)TMCs show large grain size, uniform surface morphology, high hole mobility (up to 142 cm(2)V(-1)s(-1)), as well as low trap (defect) densities. These properties suggest that TMCs can effectively suppress the radiative and nonradiative recombination loss, thus provide a promising way for maximizing the efficiency of perovskite solar cells.
DOI	10.1002/aenm.202000453
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收录类别	SCI ; EI
语种	英语
引用统计
文献类型	期刊论文
条目标识符	http://ir.ciomp.ac.cn/handle/181722/64990
专题	中国科学院长春光学精密机械与物理研究所
推荐引用方式 GB/T 7714	W. C. Kong,S. W. Wang,F. Li,et al. Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance[J]. Advanced Energy Materials,2020,10(34):8.
APA	W. C. Kong.,S. W. Wang.,F. Li.,C. Zhao.,J. Xing.,...&W. L. Yu and C. L. Guo.(2020).Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance.Advanced Energy Materials,10(34),8.
MLA	W. C. Kong,et al."Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance".Advanced Energy Materials 10.34(2020):8.

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