Self-cleaning semiconductor heterojunction substrate: ultrasensitive detection and photocatalytic degradation of organic pollutants for environmental remediation

doi:10.1038/s41378-020-00222-1

CIOMP OpenIR

	Self-cleaning semiconductor heterojunction substrate: ultrasensitive detection and photocatalytic degradation of organic pollutants for environmental remediation
	M. Y. Hu,Y. N. Quan,S. Yang,R. Su,H. L. Liu,M. Gao,L. Chen and J. H. Yang
	2020
发表期刊	Microsystems & Nanoengineering
ISSN	2055-7434
卷号	6 期号:1 页码:10
摘要	Emerging technologies in the field of environmental remediation are becoming increasingly significant owing to the increasing demand for eliminating significant amounts of pollution in water, soil, and air. We designed and synthesized MoS2/Fe2O3 heterojunction nanocomposites (NCs) as multifunctional materials that are easily separated and reused. The trace detection performance of the prepared sample was examined using bisphenol A (BPA) as the probe molecule, with limits of detection as low as 10(-9)M; this detection limit is the lowest among all reported semiconductor substrates. BPA was subjected to rapid photocatalytic degradation by MoS2/Fe2O3 NCs under ultraviolet irradiation. The highly recyclable MoS2/Fe2O3 NCs exhibited photo-Fenton catalytic activity for BPA and good detection ability when reused as a surface-enhanced Raman scattering (SERS) substrate after catalysis. The SERS and photocatalysis mechanisms were proposed while considering the effects of the Z-scheme charge-transfer paths, three-dimensional flower-like structures, and dipole-dipole coupling. Moreover, the prepared MoS2/Fe2O3 NCs were successfully applied in the detection of BPA in real lake water and milk samples. Herein, we present insights into the development of MoS2/Fe2O3 materials, which can be used as multifunctional materials in chemical sensors and in photocatalytic wastewater treatments for the removal of recalcitrant organic pollutants. Nanomaterials: environmental remediationPhotocatalytic MoS2/Fe2O3 heterojunction nanocomposites are able to remove organic pollutants from wastewater under ultraviolet light. Material systems are needed that can remove organic pollutants from the environment, many of which are driven by photocatalysis. As well as the challenge of efficiently removing contaminants from the environment, the photocatalytic material must also be recovered afterwards. Here, a team led by Jinghai Yang from Jilin Normal University report a MoS2/Fe2O3 nanocomposite that photocatalytically degrades bisphenol A under ultraviolet irradiation. Their semiconducting composite can also function as an effective SERS catalysis for bisphenol A. Compared to the component materials - MoS2 and Fe2O3 - the rate of degradation and sensitivity of the nanocomposite were both enhanced, and could be recovered from a solution via the use of a magnetic field.
DOI	10.1038/s41378-020-00222-1
URL	查看原文
收录类别	SCI ; EI
语种	英语
引用统计
文献类型	期刊论文
条目标识符	http://ir.ciomp.ac.cn/handle/181722/64872
专题	中国科学院长春光学精密机械与物理研究所
推荐引用方式 GB/T 7714	M. Y. Hu,Y. N. Quan,S. Yang,R. Su,H. L. Liu,M. Gao,L. Chen and J. H. Yang. Self-cleaning semiconductor heterojunction substrate: ultrasensitive detection and photocatalytic degradation of organic pollutants for environmental remediation[J]. Microsystems & Nanoengineering,2020,6(1):10.
APA	M. Y. Hu,Y. N. Quan,S. Yang,R. Su,H. L. Liu,M. Gao,L. Chen and J. H. Yang.(2020).Self-cleaning semiconductor heterojunction substrate: ultrasensitive detection and photocatalytic degradation of organic pollutants for environmental remediation.Microsystems & Nanoengineering,6(1),10.
MLA	M. Y. Hu,Y. N. Quan,S. Yang,R. Su,H. L. Liu,M. Gao,L. Chen and J. H. Yang."Self-cleaning semiconductor heterojunction substrate: ultrasensitive detection and photocatalytic degradation of organic pollutants for environmental remediation".Microsystems & Nanoengineering 6.1(2020):10.

条目包含的文件
文件名称/大小	文献类型	版本类型	开放类型	使用许可
Hu-2020-Self-cleanin（3818KB）	期刊论文	出版稿	开放获取	CC BY-NC-SA	浏览请求全文