Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %

doi:10.1016/j.nanoen.2019.104224

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	Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %
	F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei
	2020
发表期刊	Nano Energy
ISSN	2211-2855
卷号	67 页码:8
摘要	The quality of the photoactive film is a significant factor in determining the power conversion efficiency (PCE) and the stability of pemvskite solar cells (PSCs). We report a simple upgraded antisolvent washing treatment using iodine modulation, which significantly improves the MAPbI(3) films with high crystallinity and chemical uniformity. A detailed model for improving the mechanism is proposed to describe how the upgraded antisolvent enhances both the perovskite crystallization and passivates the under-coordinated Pb2+ dangling bond. PSCs fabricated with the FTO/TiO2/MAPbI(3)/Spiro-OMeTAD/Ag architecture used high quality films with less defective surfaces, present a PCE of 21.33%, retaining 91% of its initial value in ambient without any encapsulation after 30 days. These results provide insight into the surface defect passivation process achieved by halide ions balance while providing a simple and efficient process that can be extensively used to fabricate high-quality perovskite films.
DOI	10.1016/j.nanoen.2019.104224
URL	查看原文
收录类别	SCI ; EI
语种	英语
引用统计	被引频次：47[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.ciomp.ac.cn/handle/181722/64631
专题	中国科学院长春光学精密机械与物理研究所
推荐引用方式 GB/T 7714	F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei. Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %[J]. Nano Energy,2020,67:8.
APA	F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei.(2020).Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %.Nano Energy,67,8.
MLA	F. Y. Wang,M. F. Yang,S. Yang,X. Qu,L. L. Yang,L. Fan,J. H. Yang and F. Rosei."Iodine-assisted antisolvent engineering for stable perovskite solar cells with efficiency >21.3 %".Nano Energy 67(2020):8.

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