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A Highly Sensitive Single Crystal Perovskite-Graphene Hybrid Vertical Photodetector
Y. T. Zou,T. T. Zou,C. Zhao,B. Wang,J. Xing,Z. Yu,J. L. Cheng,W. Xin,J. J. Yang,W. L. Yu,H. L. Dong and C. L. Guo
2020
发表期刊Small
ISSN1613-6810
卷号16期号:25页码:9
摘要Organolead trihalide perovskites have attracted significant attention for optoelectronic applications due to their excellent physical properties in the past decade. Generally, both grain boundaries in perovskite films and the device structure play key roles in determining the device performance, especially for horizontal-structured device. Here, the first optimized vertical-structured photodetector with the perovskite single crystal MAPbBr(3) as the light absorber and graphene as the transport layer is shown. The hybrid device combines strong photoabsorption characteristics of perovskite and high carrier mobility of flexible graphene, exhibits excellent photoresponse performance with high photoresponsivity (approximate to 1017.1 A W-1) and high photodetectivity (approximate to 2.02 x 10(13) Jones) in a low light intensity (0.66 mW cm(-2)) under the actuations of 3 V bias and laser irradiation at 532 nm. In particular, an ultrahigh photoconductive gain of approximate to 2.37 x 10(3) is attained because of fast charge transfer in the graphene and large recombination lifetime in the perovskite single crystal. The vertical architecture combining perovskite crystal with highly conductive graphene offers opportunities to fulfill the synergistic effect of perovskite and 2D materials, is thus promising for developing high-performance electronic and optoelectronic devices.
DOI10.1002/smll.202000733
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收录类别SCI
语种英语
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被引频次:54[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/64565
专题中国科学院长春光学精密机械与物理研究所
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GB/T 7714
Y. T. Zou,T. T. Zou,C. Zhao,B. Wang,J. Xing,Z. Yu,J. L. Cheng,W. Xin,J. J. Yang,W. L. Yu,H. L. Dong and C. L. Guo. A Highly Sensitive Single Crystal Perovskite-Graphene Hybrid Vertical Photodetector[J]. Small,2020,16(25):9.
APA Y. T. Zou,T. T. Zou,C. Zhao,B. Wang,J. Xing,Z. Yu,J. L. Cheng,W. Xin,J. J. Yang,W. L. Yu,H. L. Dong and C. L. Guo.(2020).A Highly Sensitive Single Crystal Perovskite-Graphene Hybrid Vertical Photodetector.Small,16(25),9.
MLA Y. T. Zou,T. T. Zou,C. Zhao,B. Wang,J. Xing,Z. Yu,J. L. Cheng,W. Xin,J. J. Yang,W. L. Yu,H. L. Dong and C. L. Guo."A Highly Sensitive Single Crystal Perovskite-Graphene Hybrid Vertical Photodetector".Small 16.25(2020):9.
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