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Charge transfer dynamics in a singlet fission organic molecule and organometal perovskite bilayer structure
D. Q. Guo,L. Ma,Z. L. Zhou,D. B. Lin,C. Wang,X. Zhao,F. T. Zhang,J. H. Zhang and Z. G. Nie
2020
发表期刊Journal of Materials Chemistry A
ISSN2050-7488
卷号8期号:11页码:5572-5579
摘要Carrier dynamics between singlet fission molecules and a perovskite were studied using transient absorption measurements on TIPS-pentacene/CH3NH3PbI3 (MAPbI(3)) bilayer, pristine MAPbI(3) and TIPS-pentacene films. Ultrafast electron transfer within 1.5 ps is verified to proceed directly from the correlated bound triplet pair states of TIPS-pentacene generated by a singlet fission process to the MAPbI(3) conduction band. Hole transfer from MAPbI(3) to TIPS-pentacene proceeds on a much longer time scale of tens of ns. Our study not only unveils the charge carrier dynamics in a singlet fission molecule/perovskite bilayer structure, but also provides new insights on the design of singlet fission sensitized perovskite solar cells with enhanced performance.
DOI10.1039/c9ta11022d
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收录类别SCI
语种英语
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文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/64357
专题中国科学院长春光学精密机械与物理研究所
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D. Q. Guo,L. Ma,Z. L. Zhou,D. B. Lin,C. Wang,X. Zhao,F. T. Zhang,J. H. Zhang and Z. G. Nie. Charge transfer dynamics in a singlet fission organic molecule and organometal perovskite bilayer structure[J]. Journal of Materials Chemistry A,2020,8(11):5572-5579.
APA D. Q. Guo,L. Ma,Z. L. Zhou,D. B. Lin,C. Wang,X. Zhao,F. T. Zhang,J. H. Zhang and Z. G. Nie.(2020).Charge transfer dynamics in a singlet fission organic molecule and organometal perovskite bilayer structure.Journal of Materials Chemistry A,8(11),5572-5579.
MLA D. Q. Guo,L. Ma,Z. L. Zhou,D. B. Lin,C. Wang,X. Zhao,F. T. Zhang,J. H. Zhang and Z. G. Nie."Charge transfer dynamics in a singlet fission organic molecule and organometal perovskite bilayer structure".Journal of Materials Chemistry A 8.11(2020):5572-5579.
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