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Balanced strain-dependent carrier dynamics in flexible organic-inorganic hybrid perovskites
C. Wang, L. Ma, D. A. Guo, X. Zhao, Z. L. Zhou, D. B. Lin, F. T. Zhang, W. R. Zhao, J. H. Zhang and Z. G. Nie
2020
发表期刊Journal of Materials Chemistry C
ISSN2050-7526
卷号8期号:10页码:3374-3379
摘要Carrier dynamics of flexible organic-inorganic hybrid perovskite CH3NH3PbI3 (MAPbI(3)) films under various strains after photoexcitation were characterized by using time-resolved spectroscopy. The time-resolved photoluminescence study demonstrated that the charge carrier lifetime increases with increasing tensile strain, while it decreases with increasing compressive strain. This balanced optical response to tensile and compressive strains sheds light on the origin of ultra-stable optoelectric properties and overall film flexibility performance, which is further corroborated by transient absorption measurements. Moreover, the stability of flexible MAPbI(3) films was enhanced by doping a tiny amount of rubrene molecules in an MAPbI(3) precursor, without influencing the film structure or carrier dynamics. Our study provides new insights into the outstanding optoelectric properties and flexibility of the films and offers a novel method to improve the stability of organic-inorganic hybrid perovskite based flexible devices.
DOI10.1039/c9tc05763c
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收录类别SCI
语种英语
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文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/64328
专题中国科学院长春光学精密机械与物理研究所
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GB/T 7714
C. Wang, L. Ma, D. A. Guo, X. Zhao, Z. L. Zhou, D. B. Lin, F. T. Zhang, W. R. Zhao, J. H. Zhang and Z. G. Nie. Balanced strain-dependent carrier dynamics in flexible organic-inorganic hybrid perovskites[J]. Journal of Materials Chemistry C,2020,8(10):3374-3379.
APA C. Wang, L. Ma, D. A. Guo, X. Zhao, Z. L. Zhou, D. B. Lin, F. T. Zhang, W. R. Zhao, J. H. Zhang and Z. G. Nie.(2020).Balanced strain-dependent carrier dynamics in flexible organic-inorganic hybrid perovskites.Journal of Materials Chemistry C,8(10),3374-3379.
MLA C. Wang, L. Ma, D. A. Guo, X. Zhao, Z. L. Zhou, D. B. Lin, F. T. Zhang, W. R. Zhao, J. H. Zhang and Z. G. Nie."Balanced strain-dependent carrier dynamics in flexible organic-inorganic hybrid perovskites".Journal of Materials Chemistry C 8.10(2020):3374-3379.
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