Changchun Institute of Optics,Fine Mechanics and Physics,CAS
Third harmonic generation of undoped graphene in Hartree-Fock approximation | |
J.L.Cheng; J.E.Sipe; C.L.Guo | |
2019 | |
发表期刊 | Physical Review B
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ISSN | 2469-9950 |
卷号 | 100期号:24页码:8 |
摘要 | We theoretically investigate the effects of Coulomb interaction, at the level of the unscreened Hartree-Fock approximation in an equation of motion framework, on third harmonic generation from undoped graphene. The unperturbed electronic states are described by a widely used two-band tight-binding model and the Coulomb interaction is described by the Ohno potential. The ground state is renormalized by taking into account the Hartree-Fock term and the optical conductivities are obtained by numerically solving the equations of motion. The absolute values of conductivity for third-harmonic generation depend on the photon frequency Omega as Omega(-n) for h Omega < 1, and then show a peak as 3h Omega approaches the renormalized energy of the M point. Taking into account the Coulomb interaction, n is found to be 5.5, which is significantly greater than the value of 4 found with the neglect of the Coulomb interaction. Therefore, the Coulomb interaction enhances third-harmonic generation at low photon energies-for our parameters h Omega < 0.8 eV-and then reduces it until the photon energy reaches about 2.1 eV. The effect of the background dielectric constant is also considered. |
关键词 | Materials Science,Physics |
DOI | 10.1103/PhysRevB.100.245433 |
URL | 查看原文 |
收录类别 | SCI ; EI |
语种 | 英语 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ciomp.ac.cn/handle/181722/63436 |
专题 | 中国科学院长春光学精密机械与物理研究所 |
推荐引用方式 GB/T 7714 | J.L.Cheng,J.E.Sipe,C.L.Guo. Third harmonic generation of undoped graphene in Hartree-Fock approximation[J]. Physical Review B,2019,100(24):8. |
APA | J.L.Cheng,J.E.Sipe,&C.L.Guo.(2019).Third harmonic generation of undoped graphene in Hartree-Fock approximation.Physical Review B,100(24),8. |
MLA | J.L.Cheng,et al."Third harmonic generation of undoped graphene in Hartree-Fock approximation".Physical Review B 100.24(2019):8. |
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