Changchun Institute of Optics,Fine Mechanics and Physics,CAS
Pressure-induced K-Λ Crossover of Excitons Emissions in Monolayer WSe2 and MoSe2 | |
Fu, Xin-Peng; Zhou, Qiang; Qin, Li; Li, Fang-Fei; Fu, Xi-Hong | |
2018 | |
发表期刊 | CHINESE JOURNAL OF LUMINESCENCE |
ISSN | 10007032 |
卷号 | 39期号:12页码:1647-1653 |
摘要 | Monolayer MoSe2 and WSe2 samples were prepared by mechanical exfoliation in diamond anvil cell(DAC). The high-pressure micro-area fluorescence spectroscopy technique was used to study excitons emission behavior under pressure in argon pressure-transmitting medium(PTM). The neutral and negative exciton evolutionary trends of monolayer WSe2 showed an inflection point at 2.43 GPa, and the neutral exciton emission of monolayer MoSe2 appeared a new split peak at 3.7 GPa. Combined with the first-principles calculation and analysis, we confirmed that the mechanism of these discontinuities is the pressure-induced conduction band bottom K- crossover. This result can be extended to the entire two-dimensional layered material family, and laying foundation for the development of exciton devices. 2018, Science Press. All right reserved. |
关键词 | Tungsten compounds Calculations Excitons Fluorescence spectroscopy Molybdenum compounds Monolayers Selenium compounds |
DOI | 10.3788/fgxb20183912.1647 |
收录类别 | EI |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ciomp.ac.cn/handle/181722/60776 |
专题 | 中国科学院长春光学精密机械与物理研究所 |
推荐引用方式 GB/T 7714 | Fu, Xin-Peng,Zhou, Qiang,Qin, Li,et al. Pressure-induced K-Λ Crossover of Excitons Emissions in Monolayer WSe2 and MoSe2[J]. CHINESE JOURNAL OF LUMINESCENCE,2018,39(12):1647-1653. |
APA | Fu, Xin-Peng,Zhou, Qiang,Qin, Li,Li, Fang-Fei,&Fu, Xi-Hong.(2018).Pressure-induced K-Λ Crossover of Excitons Emissions in Monolayer WSe2 and MoSe2.CHINESE JOURNAL OF LUMINESCENCE,39(12),1647-1653. |
MLA | Fu, Xin-Peng,et al."Pressure-induced K-Λ Crossover of Excitons Emissions in Monolayer WSe2 and MoSe2".CHINESE JOURNAL OF LUMINESCENCE 39.12(2018):1647-1653. |
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