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Strong third-order optical nonlinearities of Ag nanoparticles synthesized by laser ablation of bulk silver in water and air
Boltaev, G. S.1; Ganeev, R. A.1; Krishnendu, P. S.1; Maurya, S. K.1; Redkin, P. V.1; Rao, K. S.1; Zhang, K.1; Guo, Chunlei1,2
2018-11-01
Source PublicationAPPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING
ISSN0947-8396
Volume124Issue:11Pages:15
Corresponding AuthorGaneev, R. A.(rashid_ganeev@mail.ru)
AbstractWe demonstrate the correlation between strong nonlinear optical response of silver nanoparticles (Ag NPs) out of plasmon resonance and efficient third harmonic generation in the plasmas containing Ag NPs. The dynamics of nonlinear optical response of the 8nm and 50nm Ag NPs prepared by laser ablation of bulk silver in deionized water using 6ns, 200ps, and 60fs laser pulses is systematically analyzed. Their optical limiting properties are studied at the wavelengths of 800 and 355nm, using femtosecond and nanosecond laser pulses. Nonlinear absorption coefficient of 8nm Ag NPs at the wavelength of 1064nm was measured to be as high as 3x10(-5)cmW(-1). Nonlinear refraction shows the change of sign with variation of the wavelength and duration of probe laser pulses. The theoretical calculation of silver ablation shows the formation of a few nanometer sized particles. We also analyze third harmonic generation in the laser-produced plasmas containing Ag NPs and attribute the enhancement of this process to the influence of small silver clusters. The conversion efficiency of 800nm towards the third harmonic was measured to be 4x10(-3), which was a few times larger compared with similar process in air.
Keywordharmonic-generation size femtosecond absorption dynamics responses ethanol liquids pulses order Materials Science Physics
DOI10.1007/s00339-018-2195-z
WOS KeywordHARMONIC-GENERATION ; SIZE ; FEMTOSECOND ; ABSORPTION ; DYNAMICS ; RESPONSES ; ETHANOL ; LIQUIDS ; PULSES ; ORDER
Indexed BySCI
Language英语
Funding ProjectNatural Science Foundation of China[61774155] ; Natural Science Foundation of China[61705227] ; National Key Research and Development Program of China[2017YFB1104700]
Funding OrganizationNatural Science Foundation of China ; National Key Research and Development Program of China
WOS Research AreaMaterials Science ; Physics
WOS SubjectMaterials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000447991200003
PublisherSPRINGER HEIDELBERG
Citation statistics
Cited Times:8[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.ciomp.ac.cn/handle/181722/60404
Collection中国科学院长春光学精密机械与物理研究所
Corresponding AuthorGaneev, R. A.
Affiliation1.Chinese Acad Sci, Changchun Inst Opt Fine Mech & Phys, State Key Lab Appl Opt, Guo China US Photon Lab, Changchun 130033, Jilin, Peoples R China
2.Univ Rochester, Inst Opt, Rochester, NY 14627 USA
Recommended Citation
GB/T 7714
Boltaev, G. S.,Ganeev, R. A.,Krishnendu, P. S.,et al. Strong third-order optical nonlinearities of Ag nanoparticles synthesized by laser ablation of bulk silver in water and air[J]. APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING,2018,124(11):15.
APA Boltaev, G. S..,Ganeev, R. A..,Krishnendu, P. S..,Maurya, S. K..,Redkin, P. V..,...&Guo, Chunlei.(2018).Strong third-order optical nonlinearities of Ag nanoparticles synthesized by laser ablation of bulk silver in water and air.APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING,124(11),15.
MLA Boltaev, G. S.,et al."Strong third-order optical nonlinearities of Ag nanoparticles synthesized by laser ablation of bulk silver in water and air".APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING 124.11(2018):15.
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