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Synthesis of Fe3O4@SiO2@ZnO-Ag core-shell microspheres for the repeated photocatalytic degradation of rhodamine B under UV irradiation
Wang, J.; J. H. Yang; X. Y. Li; B. Wei; D. D. Wang; H. Song; H. J. Zhai and X. F. Li
2015
发表期刊Journal of Molecular Catalysis a-Chemical
卷号406页码:97-105
摘要Herein, novel Fe3O4@SiO2@ZnO-Ag core-shell microstructures were synthesized through template synthesis and layer-by-layer deposition. The obtained samples were characterized in terms of morphology, composition, optical and magnetic property by various analytical techniques and subsequently tested for the photocatalytic activities. In comparison with Fe3O4@SiO2@ZnO, the as-obtained multi-shelled Fe3O4@SiO2@ZnO-Ag hierarchical microspheres exhibit a significant enhanced photocatalytic activity toward the photodegradation of Rhodamine B (RhB) aqueous solution under UV light. The enhanced photocatalytic activities of the core-shell photocatalyst are primarily ascribed to the reduced recombination probability of photogenerated electrons/holes in the surface of hierarchical microspheres. Moreover, the hierarchical microstructured Fe3O4@SiO2@ZnO-Ag photocatalysts could be easily collected and separated by using a magnetic field and reused without any appreciable decrease on photocatalytic efficiency after running six times. The enhanced photocatalytic performance and magnetic recyclability, in combination with the superior chemical stability, make these multifunctional microstructures promising candidates to eliminate aquatic contaminants and meet the demands of future environmental issues. (C) 2015 Elsevier B.V. All rights reserved.
收录类别SCI
文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/55467
专题中科院长春光机所知识产出
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Wang, J.,J. H. Yang,X. Y. Li,et al. Synthesis of Fe3O4@SiO2@ZnO-Ag core-shell microspheres for the repeated photocatalytic degradation of rhodamine B under UV irradiation[J]. Journal of Molecular Catalysis a-Chemical,2015,406:97-105.
APA Wang, J..,J. H. Yang.,X. Y. Li.,B. Wei.,D. D. Wang.,...&H. J. Zhai and X. F. Li.(2015).Synthesis of Fe3O4@SiO2@ZnO-Ag core-shell microspheres for the repeated photocatalytic degradation of rhodamine B under UV irradiation.Journal of Molecular Catalysis a-Chemical,406,97-105.
MLA Wang, J.,et al."Synthesis of Fe3O4@SiO2@ZnO-Ag core-shell microspheres for the repeated photocatalytic degradation of rhodamine B under UV irradiation".Journal of Molecular Catalysis a-Chemical 406(2015):97-105.
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