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Fabrication, characterization and application of Cu2ZnSn(S,Se)(4) absorber layer via a hybrid ink containing ball milled powders
Li, C. R.; B. Yao; Y. F. Li; Z. Y. Xiao; Z. H. Ding; H. F. Zhao; L. G. Zhang and Z. Z. Zhang
2015
发表期刊Journal of Alloys and Compounds
卷号643页码:152-158
摘要Cu2ZnSnS4 (CZTS) powder with kesterite structure was prepared by ball milling of mixture of Cu2S, ZnS and SnS2 powders for more than 15 h. By dispersing the milled CZTS powder in a Cu-, Zn- and Sn-chalcogenide precursor solution, a hybrid ink was fabricated. With the hybrid ink, a precursor CZTS film was deposited on Mo coated soda-lime glass by spin-coating. In order to obtain Cu2ZnSn(S,Se)(4) (CZTSSe) absorber film with kesterite structure, the CZTS film was annealed at 560 degrees C for 15 min in Se ambient. It is demonstrated that the annealed film is dominated by a thick layer of kesterite CZTSSe with larger grain size and Cu8Fe3Sn2(S,Se)(12) impurity phase with the exception of a very thin layer of kesterite CZTS with smaller grain size at interface between the CZTSSe and Mo layers. Solar cell device was fabricated by using the annealed CZTSSe film as absorber layer, and its conversion efficiency reached 4.2%. Mechanism of formation of the kesterite CZTS powder and CZTSSe film as well as effect of impurity phases on conversion efficiency are discussed in the present paper. The present results suggest that the hybrid ink approach combining with ball milling is a simple, low cost and promising method for preparation of kesterite CZTSSe absorber film and CZTSSe-based solar cell. (C) 2015 Elsevier B.V. All rights reserved.
收录类别SCI
文献类型期刊论文
条目标识符http://ir.ciomp.ac.cn/handle/181722/55309
专题中科院长春光机所知识产出
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Li, C. R.,B. Yao,Y. F. Li,et al. Fabrication, characterization and application of Cu2ZnSn(S,Se)(4) absorber layer via a hybrid ink containing ball milled powders[J]. Journal of Alloys and Compounds,2015,643:152-158.
APA Li, C. R..,B. Yao.,Y. F. Li.,Z. Y. Xiao.,Z. H. Ding.,...&L. G. Zhang and Z. Z. Zhang.(2015).Fabrication, characterization and application of Cu2ZnSn(S,Se)(4) absorber layer via a hybrid ink containing ball milled powders.Journal of Alloys and Compounds,643,152-158.
MLA Li, C. R.,et al."Fabrication, characterization and application of Cu2ZnSn(S,Se)(4) absorber layer via a hybrid ink containing ball milled powders".Journal of Alloys and Compounds 643(2015):152-158.
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