Changchun Institute of Optics,Fine Mechanics and Physics,CAS
Self-assembled hierarchical Bi12TiO20-graphene nanoarchitectures with excellent simulated sunlight photocatalytic activity | |
Guo W.; Yang Y. X.; Guo Y. N.; Jia Y. Q.; Liu H. B.; Guo Y. H. | |
2014 | |
发表期刊 | Physical Chemistry Chemical Physics
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ISSN | ISBN/1463-9076 |
卷号 | 16期号:6页码:2705-2714 |
摘要 | A series of hierarchical Bi12TiO20-graphene nanoarchitectures (Bi12TiO20-GR) with GR loadings from 1% to 10% are fabricated by a single-step solvothermal treatment technique, and the intimate interfacial contact between flexible GR sheets and flower-like Bi12TiO20 nanocrystals is observed in the Bi12TiO20-GR composites. As a novel composite photocatalyst, Bi12TiO20-GR with GR loading of 2% possesses the highest simulated sunlight photocatalytic activity towards the degradation of two typical organic pollutants, methyl orange (MO) and p-nitrophenol (PNP). Furthermore, the separation and transportation of the photogenerated carriers in the simulated sunlight-irradiating Bi12TiO20-GR system is studied, meanwhile, the active species (h(VB)(+), O-2(center dot-) and center dot OH) generated in the Bi12TiO20-GR-photocatalyzed PNP degradation system are identified by free radical and hole scavenging experiments. Based on the experimental and theoretical results, the mechanism and pathway of photocatalytic degradation of PNP in the simulated sunlight-irradiating Bi12TiO20-GR system are proposed. |
收录类别 | SCI |
语种 | 英语 |
文献类型 | 期刊论文 |
条目标识符 | http://ir.ciomp.ac.cn/handle/181722/44361 |
专题 | 中科院长春光机所知识产出 |
推荐引用方式 GB/T 7714 | Guo W.,Yang Y. X.,Guo Y. N.,et al. Self-assembled hierarchical Bi12TiO20-graphene nanoarchitectures with excellent simulated sunlight photocatalytic activity[J]. Physical Chemistry Chemical Physics,2014,16(6):2705-2714. |
APA | Guo W.,Yang Y. X.,Guo Y. N.,Jia Y. Q.,Liu H. B.,&Guo Y. H..(2014).Self-assembled hierarchical Bi12TiO20-graphene nanoarchitectures with excellent simulated sunlight photocatalytic activity.Physical Chemistry Chemical Physics,16(6),2705-2714. |
MLA | Guo W.,et al."Self-assembled hierarchical Bi12TiO20-graphene nanoarchitectures with excellent simulated sunlight photocatalytic activity".Physical Chemistry Chemical Physics 16.6(2014):2705-2714. |
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